At a news briefing, they confirmed that Younes Abouyaaqoub, 22, was suspected of driving the van which ploughed into dozens of people, killing 13.
CCTV footage in Spanish media appears to show him walking through a market district shortly after the attack.
A manhunt has been extended across Europe and police say he may be armed.
Some 90 minutes after mowing down dozens of people on the central Las Ramblas avenue, Abouyaaqoub fled to the city's university district, police say.
Abouyaaqoub is alleged to have hijacked the car before driving it through a police checkpoint and later abandoning the vehicle. Police say he may have crossed into France.
The male driver of the car, Pau PĂ©rez, 34, from Vila Franca, was found stabbed to death in the back seat, becoming the 15th victim of the Barcelona bloodshed and a later attack in the resort of Cambrils.
A woman died in Cambrils when a car was driven into pedestrians, and five suspected jihadists were killed at the scene by police.
At a news conference on Monday, officials also revealed there were "strong indications" that an imam suspected of radicalising the young men who carried out the attacks had died in an explosion at a house in Alcanar, south of Barcelona, that was being used as a bomb factory.
Source: BBC
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